Amstruplamb4739

We investigate the differential ionization probability of chiral molecules in the strong-field regime as a function of the helicity of the incident light. To this end, we analyze the fourfold ionization of bromochlorofluoromethane (CHBrClF) with subsequent fragmentation into four charged fragments and different dissociation channels of the singly ionized methyloxirane. Selleck Bevacizumab By resolving for the molecular orientation, we show that the photoion circular dichroism signal strength is increased by 2 orders of magnitude.Glasses, unlike their crystalline counterparts, exhibit low-frequency nonphononic excitations whose frequencies ω follow a universal D(ω)∼ω^4 density of states. The process of glass formation generates positional disorder intertwined with mechanical frustration, posing fundamental challenges in understanding the origins of glassy nonphononic excitations. Here we suggest that minimal complexes-mechanically frustrated and positionally disordered local structures-embody the minimal physical ingredients needed to generate glasslike excitations. We investigate the individual effects of mechanical frustration and positional disorder on the vibrational spectrum of isolated minimal complexes, and demonstrate that ensembles of marginally stable minimal complexes yield D(ω)∼ω^4. Furthermore, glasslike excitations emerge by embedding a single minimal complex within a perfect lattice. Consequently, minimal complexes offer a conceptual framework to understand glasslike excitations from first principles, as well as a practical computational method for introducing them into solids.Precise knowledge of the charge and rigidity dependence of the secondary cosmic ray fluxes and the secondary-to-primary flux ratios is essential in the understanding of cosmic ray propagation. We report the properties of heavy secondary cosmic ray fluorine F in the rigidity R range 2.15 GV to 2.9 TV based on 0.29 million events collected by the Alpha Magnetic Spectrometer experiment on the International Space Station. The fluorine spectrum deviates from a single power law above 200 GV. The heavier secondary-to-primary F/Si flux ratio rigidity dependence is distinctly different from the lighter B/O (or B/C) rigidity dependence. In particular, above 10 GV, the F/Si/B/O ratio can be described by a power law R^δ with δ=0.052±0.007. This shows that the propagation properties of heavy cosmic rays, from F to Si, are different from those of light cosmic rays, from He to O, and that the secondary cosmic rays have two classes.Under uniaxial shock compression, the steepness of the plastic shock front usually exhibits power law characteristics with the Hugoniot pressure, also known as the "Swegle-Grady law." In this Letter, we show that the Swegle-Grady law can be described better by a third power law rather than the classical fourth power law at the strain rate between 10^5-10^7  s^-1. A simple dislocation-based continuum model is developed, which reproduced the third power law and revealed very good agreement with recent experiments of multiple types of metals quantitatively. New insights into this unusual macroscopic phenomenon are presented through quantifying the connection between the macroscopic mechanical response and the collective dynamics of dislocation assembles. It is found that the Swegle-Grady law results from the particular stress dependence of the plasticity behaviors, and that the difference between the third power scaling and the classical fourth power scaling results from different shock dissipative actions.Mesoscopic conductance fluctuations are a ubiquitous signature of phase-coherent transport in small conductors, exhibiting universal character independent of system details. In this Letter, however, we demonstrate a pronounced breakdown of this universality, due to the interplay of local and remote phenomena in transport. Our experiments are performed in a graphene-based interaction-detection geometry, in which an artificial magnetic texture is induced in the graphene layer by covering a portion of it with a micromagnet. When probing conduction at some distance from this region, the strong influence of remote factors is manifested through the appearance of giant conductance fluctuations, with amplitude much larger than e^2/h. This violation of one of the fundamental tenets of mesoscopic physics dramatically demonstrates how local considerations can be overwhelmed by remote signatures in phase-coherent conductors.A major challenge in developing quantum computing technologies is to accomplish high precision tasks by utilizing multiplex optimization approaches, on both the physical system and algorithm levels. Loss functions assessing the overall performance of quantum circuits can provide the foundation for many optimization techniques. In this Letter, we use the quadratic error loss and the final-state fidelity loss to characterize quantum circuits. We find that the distribution of computation error is approximately Gaussian, which in turn justifies the quadratic error loss. It is shown that these loss functions can be efficiently evaluated in a scalable way by sampling from Clifford-dominated circuits. We demonstrate the results by numerically simulating 10-qubit noisy quantum circuits with various error models as well as executing 4-qubit circuits with up to ten layers of 2-qubit gates on a superconducting quantum processor. Our results pave the way toward the optimization-based quantum device and algorithm design in the intermediate-scale quantum regime.Quasielastic ^12C(e,e^'p) scattering was measured at spacelike 4-momentum transfer squared Q^2=8, 9.4, 11.4, and 14.2  (GeV/c)^2, the highest ever achieved to date. Nuclear transparency for this reaction was extracted by comparing the measured yield to that expected from a plane-wave impulse approximation calculation without any final state interactions. The measured transparency was consistent with no Q^2 dependence, up to proton momenta of 8.5  GeV/c, ruling out the quantum chromodynamics effect of color transparency at the measured Q^2 scales in exclusive (e,e^'p) reactions. These results impose strict constraints on models of color transparency for protons.