Aggerholmbengtsson9736
Electrical double layers (EDLs) play a significant role in a broad range of physical phenomena related to colloidal stability, diffuse-charge dynamics, electrokinetics, and energy storage applications. Recently, it has been suggested that for large ion sizes or multivalent electrolytes, ions can arrange in a layered structure inside the EDLs. However, the widely used Poisson-Boltzmann models for EDLs are unable to capture the details of ion concentration oscillations and the effect of electrolyte valence on such oscillations. Here, by treating a pair of ions as hard spheres below the distance of closest approach and as point charges otherwise, we are able to predict ionic layering without any additional parameters or boundary conditions while still being compatible with the Poisson-Boltzmann framework. Depending on the combination of ion valence, size, and concentration, our model reveals a structured EDL with spatially oscillating ion concentrations. We report the dependence of critical ion concentration, i.e., the ion concentration above which the oscillations are observed, on the counter-ion valence and the ion size. More importantly, our model displays quantitative agreement with the results of computationally intensive models of the EDL. Finally, we analyze the nonequilibrium problem of EDL charging and demonstrate that ionic layering increases the total charge storage capacity and the charging timescale.It is well known that the acoustic properties of fluid are characterized by mass density and bulk modulus. Metafluids, the fluid metamaterials, generalize the natural fluid, which can accommodate extreme and/or negative values of these two parameters. Here, we further show that the metafluids, composed of periodic thin-walled hollow cylinders immersed in fluid, can provide not only the designable effective mass density and bulk modulus, but also a completely new effective parameter, which appears in the wave velocities as a role similar to the shear modulus of solid. The new effective parameter, describing the response of the fluid to the quadrupolar component of waves, is obtained by generalizing the effective medium theory (EMT) to include the second-order effects, which is vanishing and neglected in the conventional EMT, but giant here in the metafluids with built-in quadrupolar resonances. With the discovery of the metafluids of shearlike moduli, our Letter extends the concept of metafluids and will have a great significance in the field of metamaterials.Primordial black holes (PBHs) are a viable candidate for dark matter if the PBH masses are in the currently unconstrained "sublunar" mass range. We revisit the possibility that PBHs were produced by nucleation of false vacuum bubbles during inflation. We show that this scenario can produce a population of PBHs that simultaneously accounts for all dark matter, explains the candidate event in the Subaru Hyper Suprime-Cam (HSC) data, and contains both heavy black holes as observed by LIGO and very heavy seeds of supermassive black holes. We demonstrate with numerical studies that future observations of HSC, as well as other optical surveys, such as LSST, will be able to provide a definitive test for this generic PBH formation mechanism if it is the dominant source of dark matter.We introduce and study a novel class of sensors whose sensitivity grows exponentially with the size of the device. Remarkably, this drastic enhancement does not rely on any fine-tuning, but is found to be a stable phenomenon immune to local perturbations. Specifically, the physical mechanism behind this striking phenomenon is intimately connected to the anomalous sensitivity to boundary conditions observed in non-Hermitian topological systems. We outline concrete platforms for the practical implementation of these non-Hermitian topological sensors ranging from classical metamaterials to synthetic quantum materials.Microcavity solitons enable miniaturized coherent frequency comb sources. However, the formation of microcavity solitons can be disrupted by stimulated Raman scattering, particularly in the emerging crystalline microcomb materials with high Raman gain. MTP-131 Here, we propose and implement dissipation control-tailoring the energy dissipation of selected cavity modes-to purposely raise or lower the threshold of Raman lasing in a strongly Raman-active lithium niobate microring resonator and realize on-demand soliton mode locking or Raman lasing. Numerical simulations are carried out to confirm our analyses and agree well with experiment results. Our work demonstrates an effective approach to address strong stimulated Raman scattering for microcavity soliton generation.We analyze a quantum-classical hybrid system of steadily precessing around the fixed axis slow classical localized magnetic moments (LMMs), forming a head-to-head domain wall, surrounded by fast electrons driven out of equilibrium by LMMs and residing within a metallic wire whose connection to macroscopic reservoirs makes electronic quantum system an open one. The model captures the essence of dynamical noncollinear magnetic textures encountered in spintronics, while making it possible to obtain the exact time-dependent nonequilibrium density matrix of electronic systems and split it into four contributions. The Fermi surface contribution generates dissipative (or dampinglike in spintronics terminology) spin torque on LMMs, as the counterpart of electronic friction in nonadiabatic molecular dynamics (MD). Among two Fermi sea contributions, one generates geometric torque dominating in the adiabatic regime, which remains as the only nonzero contribution in a closed system with disconnected reservoirs. Locally geometric torque can have nondissipative (or fieldlike in spintronics terminology) component, acting as the counterpart of geometric magnetism force in nonadiabatic MD, as well as a much smaller dampinglike component acting as "geometric friction." Such current-independent geometric torque is absent from widely used micromagnetics or atomistic spin dynamics modeling of magnetization dynamics based on the Landau-Lifshitz-Gilbert equation, while previous analyses of how to include our Fermi-surface dampinglike torque have severely underestimated its total magnitude.